Helium isotopic ratios ranging from 20 to 32 times the atmospheric 3He 4He(RA) have been observed in a suite of 15 basaltic glasses from the Loihi Seamount. These ratios, which are up to four times higher than those of MORB glasses and more than twice those of nearby Kilauea, are strongly suggestive of a primitive source of volatiles supplying this volcanism. The Loihi glasses measured span a broad compositional range, and the 3He/4He ratios were found to be generally lower for the alkali basalts than for the tholeiites. The component with a lower 3He 4He ratio appears to be associated with olivine xenocrysts, within which fluid inclusions are probably the carrier of contaminant helium. One Loihi sample has a much lower isotopic ratio (