The Scituate Reservoir system is the principal drinking-water supply for more than 60 percent of the population of Rhode Island. Sodium concentrations in the reservoir have been increasing slowly in recent years despite the long-term (12 years) use of a reduced-sodium deicing agent on State-maintained highways in the reservoir drainage basin. This report identifies the major sources of sodium and chloride in the drainage basin, and assesses the relative contribution of each source to the total amounts of these constituents that entered the basin from October 1999 through September 2000 (Water Year 2000).