As a comparison to airborne infrared (IR) flux measurements, ground-based sampling of fumarole and soil gases was used to characterize the quiescent degassing of CO2 from Oldoinyo Lengai volcano. Aerial and ground-based measurements are in good agreement: ∼75% of the aerially measured CO2 flux at Lengai (0.05–0.06 × 1012 mol yr−1 or 6000–7200 tonnes CO2 d−1) can be attributed to seven large crater vents. In contrast to Etna and Vulcano Island, where 15–50% of the total CO2 flux emanates diffusely through the volcanic flanks, diffuse emissions were measured only within 500 m of the crater rim at Lengai, contributing