This dataset contains measurements of chemical concentrations of forest soil samples and associated site measurements collected in the Adirondack Ecoregion of New York State. Data are presented in four groups (tabs) in an Microsoft EXCEL 2013 spreadsheet (and comma-delimited CSV files): (1) Adirondack Sugar Maple Project (ASM), (2) Buck Creek North Watershed, (3) Buck Creek South Watershed, and (4) Western Adirondack Stream Survey (WASS) soil sampling. The ASM data were all collected in 2009 and the WASS data were all collected in 2004. The Buck Creek North Tributary Watershed was sampled in 1997 and repeated at the same plot locations in 2009/10. The Buck Creek South Tributary Watershed was sampled in 1998 and repeated at the same plot locations in 2014. Site locations (latitude, longitude) are provided in a downloadable file and dynamic ArcGIS REST service at USGS Sciencebase DOI link.