Contribution of traffic emissions to PM2.5 concentrations at bus stops in Denver, Colorado

Individuals are routinely exposed to traffic-related air pollution on their commutes, which has significant health impacts. Mitigating exposure to traffic-related pollution is a key urban sustainability concern. In Denver, Colorado, low-income Americans are more likely to rely on buses and spend time waiting at bus stops. Evaluating the contribution of traffic emissions at bus stops can provide important information on risks experienced by these populations. We measured PM_2.5 constituents at eight bus stops and one background reference site in Denver, in the summer of 2023. Source profiles, including gasoline emissions from traffic, were estimated using Positive Matrix Factorization (PMF) analysis of PM_2.5 constituents collected at a Chemical Speciation Network site in our study region. The contributions of the different sources at each bus stop were estimated by regressing the vector of species concentrations at each site (dependent variable) on the source-profile matrix from the PMF analysis (independent variables). Traffic-related emissions (~2.5–6.6 μg/m³) and secondary organics (~3–5 μg/m³) contributed to PM_2.5 at the bus stops in our dataset. The highest traffic-related emissions-derived PM_2.5 concentrations were observed at bus stops near local sources: a gas station and a car wash. The contribution of traffic-related emissions was lower at the background site (~1 μg/m³).