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Spatiotemporal patterns of mercury accumulation in lake sediments of western North America

June 28, 2016

For the Western North America Mercury Synthesis, we compiled mercury records from 165 dated sediment cores from 138 natural lakes across western North America. Lake sediments are accepted as faithful recorders of historical mercury accumulation rates, and regional and sub-regional temporal and spatial trends were analyzed with descriptive and inferential statistics. Mercury accumulation rates in sediments have increased, on average, four times (4×) from 1850 to 2000 and continue to increase by approximately 0.2 μg/m2 per year. Lakes with the greatest increases were influenced by the Flin Flon smelter, followed by lakes directly affected by mining and wastewater discharges. Of lakes not directly affected by point sources, there is a clear separation in mercury accumulation rates between lakes with no/little watershed development and lakes with extensive watershed development for agricultural and/or residential purposes. Lakes in the latter group exhibited a sharp increase in mercury accumulation rates with human settlement, stabilizing after 1950 at five times (5×) 1850 rates. Mercury accumulation rates in lakes with no/little watershed development were controlled primarily by relative watershed size prior to 1850, and since have exhibited modest increases (in absolute terms and compared to that described above) associated with (regional and global) industrialization. A sub-regional analysis highlighted that in the ecoregion Northwestern Forest Mountains, <1% of mercury deposited to watersheds is delivered to lakes. Research is warranted to understand whether mountainous watersheds act as permanent sinks for mercury or if export of “legacy” mercury (deposited in years past) will delay recovery when/if emissions reductions are achieved.

Publication Year 2016
Title Spatiotemporal patterns of mercury accumulation in lake sediments of western North America
DOI 10.1016/j.scitotenv.2016.03.167
Authors Paul Drevnick, Colin A. Cooke, Daniella Barraza, Jules M. Blais, Kenneth Coale, Brian F. Cumming, Chris Curtis, Biplob Das, William F. Donahue, Collin A. Eagles-Smith, Daniel R. Engstrom, William F. Fitzgerald, Chad V. Furl, John R. Gray, Roland I. Hall, Togwell A. Jackson, Kathleen R. Laird, W. Lyle Lockhart, Robie W. Macdonald, Alisa Mast, Callie Mathieu, Derek C.G. Muir, Peter Outridge, Scott Reinemann, Sarah E. Rothenberg, Ana Carolina Ruiz-Fernandex, V.L. St. Louis, Rhea Sanders, Hamed Sanei, Elliott Skierszkan, Peter C. Van Metre, Timothy Veverica, Johan A. Wiklund, Brent B. Wolfe
Publication Type Article
Publication Subtype Journal Article
Series Title Science of the Total Environment
Index ID 70170411
Record Source USGS Publications Warehouse
USGS Organization Forest and Rangeland Ecosystem Science Center; John Wesley Powell Center for Analysis and Synthesis; Contaminant Biology Program